National Physical Laboratory

Estimating surface effects

  Question Mark Lean

With any radiation detector only some of the emissions from a source or surface are detected. In order to estimate the activity, consideration must be given to what is present but not detected.

The active layer of the source is shown in red

A: Particle/photon emitted from surface (may or may not interact in detector)

B: Particle/photon absorbed in surface grime  (see Table 2)

C: Particle/photon absorbed in active layer (see Table 1)

D: Particle/photon back scattered from substrate (see Table 1)

E: Particle/photon absorbed in substrate.

Upper 2 emmisions

Figure 4 Schematic of emission processes from the surface of a source

Figure 4 shows what may happen to emissions that originate in the active layer of a source.  Assumptions need to be made and an account needs to be taken of the number of emissions that could not possibly be registered by the detector or in the case of (D), emissions that add to the instrument response and potentially cause an increased estimate of activity. Table 1 shows how some of these effects can be taken into account.

The surface effects illustrated can be categorised into 4 main components:
  • Geometry

4π geometry describes the emissions that occur at all angles from the nucleus. 2π geometry describes those emissions from a source that are emitted in the direction of the detector. In the case of a perfect surface, half of the emissions go up and half of them go down.

  • Backscatter

The effects of backscatter contribute to the observed reading, particularly if the contaminated surface is a high density material (for example, some floors or stainless steel workbenches). However in practice, no correction is made for this because it only affects photons and high energy betas significantly and it results in an over estimate of the activity. See Table 1.

  • Absorption in the active layer

When assessing alpha or low energy beta contamination, consideration must be given to particles that never leave the surface, i.e. self absorption. A reliable estimate of this effect can only be made if the active layer is small in relation to the range of emissions. See Table 1.

  • Absorption in surface grime

When assessing alpha or low energy beta contamination, consideration must be given to any coatings (e.g. paint or varnish) or any material that may be deposited on the contaminated surface (e.g. polish or dust) as these will absorb a proportion of the emissions. See Table 2.

By applying a correction for these surface effects to the surface activity calculated for 'ideal' contamination of this radionuclide, it is possible to estimate a more realistic value for the activity of the real contamination.

However, if the 'ideal surface' 2π detector efficiency is used, any action levels set will be too high.

Table 1 Typical correction factors

Effect Radiation affected

Magnitude of effect on the number of counts registered and how it can be accounted for

Ideal Surface

All

Multiply number of counts by 2 to account for emissions in the opposite direction to the detector


 

Non ideal surfaces

In addition to the factor of 2 above

Backscatter

High energy β

and γ

Increases surface emission by 10-20% on high atomic number backings (e.g. steel).

Reduce counts by 10-20% before multiplying by the factor of 2 for an ideal surface.

Self absorption in the active layer

Alphas

Decreases surface emission by a factor 2 or more.

Multiply counts by at least an additional factor of 2 (2 x 2 = 4) for all alphas except very thin deposits. 

Low energy βs

(0.15-0.4 MeV)

Relatively thin deposits will produce a considerable reduction in surface emission rates.

Multiply counts by at least an additional factor of 2 for all low energy betas except very thin deposits.

High energy βs

Surface emission unaffected for thin deposits 
(< 1mg cm -2)

Surface coatings

 

More details provided in Table 3

Alphas

Grime layer 5 mg cm-2 (a sheet of paper) thick totally absorbs α radiation.

Multiply by at least 2. The figure to be used rapidly approaches infinity (total absorption).

Low energy βs

Grime layer 5 mg cm-2 thick decreases surface emission by a factor of 2 or more.

Multiply counts by at least an additional factor of 2 for all low energy betas.

High energy βs

Grime layer 5 mg cm-2 thick does not significantly change surface emissions.

Table 1 Typical correction factors for absorption of radiation6

Table 2 Percentage transmission factors

Radionuclide and radiation type
238Pu 14C 36Cl 90Sr + 90Y 55Fe
Alpha Soft beta Medium beta Medium + hard beta 5.9 keV photon
Coating Mass per unit area (mg cm-2) Percentage Transmission Values

Car paint

2.6 10 50 50 95 30

Anti rust paint

4.0 0 30 90 95 35

Lacquer

2.4 10 50 90 95 50

Wood varnish

1.4 30 60 95 100 70
Furniture polish 0.1 90 95 100 100 95

Oil as applied

1.3 30 70 95 100 70

Oil wiped off

0.14 90 95 100 100 95

Grease as applied

1.8 20 60 95 100 60

The paints are one coat only. The polish is two coats. All are applied according to manufacturers’ instructions.

Table 2 Percentage transmission factors for surface coatings6

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